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Single-atom iron doped BiOCl atomic layers to promote efficient CO electroreduction towards formate

The electrocatalytic CO 2 reduction reaction to valuable fuels is a promising strategy to simultaneously tackle the crises of fossil fuel shortage and carbon emission. Herein, a single-Fe-atom was introduced into the BiOCl catalyst by a facile hydrolysis method, which exhibited a greatly enhanced ca...

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Bibliographic Details
Published in:Catalysis science & technology 2024-01, Vol.14 (1), p.62-65
Main Authors: Tian, Fengwu, Tang, Tian, Di, Xixi, Guo, Xiaosha, Liu, Dong, Shi, Yixuan, Shen, Zheng, Yu, Xiaohu, Shao, Xianzhao
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Summary:The electrocatalytic CO 2 reduction reaction to valuable fuels is a promising strategy to simultaneously tackle the crises of fossil fuel shortage and carbon emission. Herein, a single-Fe-atom was introduced into the BiOCl catalyst by a facile hydrolysis method, which exhibited a greatly enhanced catalytic performance in the electrochemical CO 2 RR to formate, exceeding 90% hydrogenation selectivity and maintaining above 90% activity for 10 hours. The electrocatalytic CO 2 reduction reaction to valuable fuels is a promising strategy to simultaneously tackle the crises of fossil fuel shortage and carbon emission.
ISSN:2044-4753
2044-4761
DOI:10.1039/d3cy01523h