Natural radioactivity in urban soils of mining centers in Armenia: Dose rate and risk assessment

Soil radioactivity levels, dose rate and radiological health risk were assessed in metal mining centers of Armenia, at the towns of Kapan and Kajaran. Archive soil samples of the multipurpose soil surveys implemented in Kapan and Kajaran were used for estimation of total alpha and total beta activit...

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Bibliographic Details
Published in:Chemosphere (Oxford) 2019-06, Vol.225, p.859-870
Main Authors: Belyaeva, Olga, Pyuskyulyan, Konstantin, Movsisyan, Nona, Saghatelyan, Armen, Carvalho, Fernando P.
Format: Article
Language:English
Subjects:
Cancer risk
Dose rate
Metal mining
Naturally occurring radioactive materials (NORM)
Total alpha/beta activity
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Summary:Soil radioactivity levels, dose rate and radiological health risk were assessed in metal mining centers of Armenia, at the towns of Kapan and Kajaran. Archive soil samples of the multipurpose soil surveys implemented in Kapan and Kajaran were used for estimation of total alpha and total beta activity levels using gas-less iMatic™ alpha/beta cօunting system (Canberra). Ten representative soil samples per town were randomly selected from different urban zones for naturally occurring radionuclide measurements (238U, 232Th, 40 K) using high purity germanium detector. Four radiological indices: radium equivalent activity, outdoor absorbed dose rate, annual effective dose equivalent and excess lifetime cancer risk were estimated based on naturally occurring radionuclide activity concentrations in soils. Results suggest that in Kapan the soil radioactivity, although enhanced by copper and gold-polymetallic mining, are not a significant risk factor to human health. In Kajaran, the soil radioactivity levels were above the background and world average values provided by UNSCEAR, but radionuclides originated in a natural geogenic source and not from mining activities. Generally, in this region no significant radiological risks were identified in relationship with molybdenum, copper, and gold-polymetallic ore mining. •Soil radioactivity enheancemet was studied based on urban geochemical survey.•Copper and polymetallic mining is the factor for natural radioactivity enheancement.•Mining legacy sites located at high altitudes preovoke NORM accumulation in vales.•Enhanced soil radioactivity due to metal mining is not risk factor to human health.
ISSN:0045-6535
1879-1298
DOI:10.1016/j.chemosphere.2019.03.057