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Environmental Levels, Sources, and Cancer Risk Assessment of PAHs Associated with PM2.5 and TSP in Monterrey Metropolitan Area
In this work, the content of polycyclic aromatic hydrocarbons (PAHs) in total suspended particles and particulate matter with an aerodynamic diameter ≤ 2.5 µm (PM 2.5 ) was analyzed using gas chromatography–mass spectrometry. In addition, a sequential chemical analysis of C-rich particles was perfor...
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| Published in: | Archives of environmental contamination and toxicology 2020-04, Vol.78 (3), p.377-391 |
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| creator | Longoria-Rodríguez, Francisco E. González, Lucy T. Mendoza, Alberto Leyva-Porras, Cesar Arizpe-Zapata, Alejandro Esneider-Alcalá, Miguel Acuña-Askar, Karim Gaspar-Ramirez, Octavio López-Ayala, Olivia Alfaro-Barbosa, Juan M. Kharissova, Oxana V. |
| description | In this work, the content of polycyclic aromatic hydrocarbons (PAHs) in total suspended particles and particulate matter with an aerodynamic diameter ≤ 2.5 µm (PM
2.5
) was analyzed using gas chromatography–mass spectrometry. In addition, a sequential chemical analysis of C-rich particles was performed through the parallel coupling of micro-Raman spectroscopy and scanning electron microscopy with X-ray scattering detection. Samples were collected at four sites in the Monterrey metropolitan area, Mexico. A total of 13 PAHs were quantified; indeno(1,2,3-
cd
)pyrene, chrysene, and benzo(
a
)anthracene were the most abundant. The total PAH concentrations at the four sampling sites ranged from 1.34 to 8.76 μg/m
3
. The diagnostic relation of the PAHs indicates that these compounds were emitted by the burning of gasoline and diesel and by the burning of charcoal and biomass. The sequential analysis correlated the morphology and the elemental/molecular composition of the C-rich particles, associated with the PAHs, with their possible emission sources. The estimated lifetime excess cancer risk for inhalation was higher than that established by the World Health Organization, which clearly makes this a potential health risk for the population. |
| doi_str_mv | 10.1007/s00244-019-00701-1 |
| format | article |
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2.5
) was analyzed using gas chromatography–mass spectrometry. In addition, a sequential chemical analysis of C-rich particles was performed through the parallel coupling of micro-Raman spectroscopy and scanning electron microscopy with X-ray scattering detection. Samples were collected at four sites in the Monterrey metropolitan area, Mexico. A total of 13 PAHs were quantified; indeno(1,2,3-
cd
)pyrene, chrysene, and benzo(
a
)anthracene were the most abundant. The total PAH concentrations at the four sampling sites ranged from 1.34 to 8.76 μg/m
3
. The diagnostic relation of the PAHs indicates that these compounds were emitted by the burning of gasoline and diesel and by the burning of charcoal and biomass. The sequential analysis correlated the morphology and the elemental/molecular composition of the C-rich particles, associated with the PAHs, with their possible emission sources. The estimated lifetime excess cancer risk for inhalation was higher than that established by the World Health Organization, which clearly makes this a potential health risk for the population.</description><identifier>ISSN: 0090-4341</identifier><identifier>EISSN: 1432-0703</identifier><identifier>DOI: 10.1007/s00244-019-00701-1</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Air pollution ; Analytical chemistry ; Anthracene ; Archives & records ; Biomass ; Biomass burning ; Burning ; Cancer ; Charcoal ; Chemical analysis ; Chemical composition ; Chrysene ; Climate change ; Correlation analysis ; Coupling (molecular) ; Diagnostic systems ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Gas chromatography ; Gasoline ; Health risks ; Industrial plant emissions ; Inhalation ; Mass spectrometry ; Mass spectroscopy ; Metropolitan areas ; Molecular weight ; Monitoring/Environmental Analysis ; Morphology ; Particulate emissions ; Particulate matter ; Pollution ; Polycyclic aromatic hydrocarbons ; Pyrene ; Raman spectroscopy ; Respiration ; Risk assessment ; Scanning electron microscopy ; Sequential analysis ; Soil Science & Conservation ; Toxicology ; Winter ; X-ray scattering</subject><ispartof>Archives of environmental contamination and toxicology, 2020-04, Vol.78 (3), p.377-391</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2020</rights><rights>Archives of Environmental Contamination and Toxicology is a copyright of Springer, (2020). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c352t-d20310406822d1b2aece84c43a799b5b3414566597207e2d0d15c3377f83ff8f3</citedby><cites>FETCH-LOGICAL-c352t-d20310406822d1b2aece84c43a799b5b3414566597207e2d0d15c3377f83ff8f3</cites><orcidid>0000-0001-6415-5296</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2378613270/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2378613270?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>315,783,787,11700,27936,27937,36072,44375,75229</link.rule.ids></links><search><creatorcontrib>Longoria-Rodríguez, Francisco E.</creatorcontrib><creatorcontrib>González, Lucy T.</creatorcontrib><creatorcontrib>Mendoza, Alberto</creatorcontrib><creatorcontrib>Leyva-Porras, Cesar</creatorcontrib><creatorcontrib>Arizpe-Zapata, Alejandro</creatorcontrib><creatorcontrib>Esneider-Alcalá, Miguel</creatorcontrib><creatorcontrib>Acuña-Askar, Karim</creatorcontrib><creatorcontrib>Gaspar-Ramirez, Octavio</creatorcontrib><creatorcontrib>López-Ayala, Olivia</creatorcontrib><creatorcontrib>Alfaro-Barbosa, Juan M.</creatorcontrib><creatorcontrib>Kharissova, Oxana V.</creatorcontrib><title>Environmental Levels, Sources, and Cancer Risk Assessment of PAHs Associated with PM2.5 and TSP in Monterrey Metropolitan Area</title><title>Archives of environmental contamination and toxicology</title><addtitle>Arch Environ Contam Toxicol</addtitle><description>In this work, the content of polycyclic aromatic hydrocarbons (PAHs) in total suspended particles and particulate matter with an aerodynamic diameter ≤ 2.5 µm (PM
2.5
) was analyzed using gas chromatography–mass spectrometry. In addition, a sequential chemical analysis of C-rich particles was performed through the parallel coupling of micro-Raman spectroscopy and scanning electron microscopy with X-ray scattering detection. Samples were collected at four sites in the Monterrey metropolitan area, Mexico. A total of 13 PAHs were quantified; indeno(1,2,3-
cd
)pyrene, chrysene, and benzo(
a
)anthracene were the most abundant. The total PAH concentrations at the four sampling sites ranged from 1.34 to 8.76 μg/m
3
. The diagnostic relation of the PAHs indicates that these compounds were emitted by the burning of gasoline and diesel and by the burning of charcoal and biomass. The sequential analysis correlated the morphology and the elemental/molecular composition of the C-rich particles, associated with the PAHs, with their possible emission sources. The estimated lifetime excess cancer risk for inhalation was higher than that established by the World Health Organization, which clearly makes this a potential health risk for the population.</description><subject>Air pollution</subject><subject>Analytical chemistry</subject><subject>Anthracene</subject><subject>Archives & records</subject><subject>Biomass</subject><subject>Biomass burning</subject><subject>Burning</subject><subject>Cancer</subject><subject>Charcoal</subject><subject>Chemical analysis</subject><subject>Chemical composition</subject><subject>Chrysene</subject><subject>Climate change</subject><subject>Correlation analysis</subject><subject>Coupling (molecular)</subject><subject>Diagnostic systems</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Gas 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Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Longoria-Rodríguez, Francisco E.</au><au>González, Lucy T.</au><au>Mendoza, Alberto</au><au>Leyva-Porras, Cesar</au><au>Arizpe-Zapata, Alejandro</au><au>Esneider-Alcalá, Miguel</au><au>Acuña-Askar, Karim</au><au>Gaspar-Ramirez, Octavio</au><au>López-Ayala, Olivia</au><au>Alfaro-Barbosa, Juan M.</au><au>Kharissova, Oxana V.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Environmental Levels, Sources, and Cancer Risk Assessment of PAHs Associated with PM2.5 and TSP in Monterrey Metropolitan Area</atitle><jtitle>Archives of environmental contamination and toxicology</jtitle><stitle>Arch Environ Contam Toxicol</stitle><date>2020-04-01</date><risdate>2020</risdate><volume>78</volume><issue>3</issue><spage>377</spage><epage>391</epage><pages>377-391</pages><issn>0090-4341</issn><eissn>1432-0703</eissn><abstract>In this work, the content of polycyclic aromatic hydrocarbons (PAHs) in total suspended particles and particulate matter with an aerodynamic diameter ≤ 2.5 µm (PM
2.5
) was analyzed using gas chromatography–mass spectrometry. In addition, a sequential chemical analysis of C-rich particles was performed through the parallel coupling of micro-Raman spectroscopy and scanning electron microscopy with X-ray scattering detection. Samples were collected at four sites in the Monterrey metropolitan area, Mexico. A total of 13 PAHs were quantified; indeno(1,2,3-
cd
)pyrene, chrysene, and benzo(
a
)anthracene were the most abundant. The total PAH concentrations at the four sampling sites ranged from 1.34 to 8.76 μg/m
3
. The diagnostic relation of the PAHs indicates that these compounds were emitted by the burning of gasoline and diesel and by the burning of charcoal and biomass. The sequential analysis correlated the morphology and the elemental/molecular composition of the C-rich particles, associated with the PAHs, with their possible emission sources. The estimated lifetime excess cancer risk for inhalation was higher than that established by the World Health Organization, which clearly makes this a potential health risk for the population.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s00244-019-00701-1</doi><tpages>15</tpages><orcidid>https://orcid.org/0000-0001-6415-5296</orcidid></addata></record> |
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| ispartof | Archives of environmental contamination and toxicology, 2020-04, Vol.78 (3), p.377-391 |
| issn | 0090-4341 1432-0703 |
| language | eng |
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| source | ABI/INFORM Global (ProQuest); Springer Link |
| subjects | Air pollution Analytical chemistry Anthracene Archives & records Biomass Biomass burning Burning Cancer Charcoal Chemical analysis Chemical composition Chrysene Climate change Correlation analysis Coupling (molecular) Diagnostic systems Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Gas chromatography Gasoline Health risks Industrial plant emissions Inhalation Mass spectrometry Mass spectroscopy Metropolitan areas Molecular weight Monitoring/Environmental Analysis Morphology Particulate emissions Particulate matter Pollution Polycyclic aromatic hydrocarbons Pyrene Raman spectroscopy Respiration Risk assessment Scanning electron microscopy Sequential analysis Soil Science & Conservation Toxicology Winter X-ray scattering |
| title | Environmental Levels, Sources, and Cancer Risk Assessment of PAHs Associated with PM2.5 and TSP in Monterrey Metropolitan Area |
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