Plugging a Molecular Wire into Photosystem I: Reconstitution of the Photoelectric Conversion System on a Gold Electrode

Plug and play: Photoinduced electron transfer occurs from photoexcited P700 in photosystem I (PSI) to a gold surface (see picture). A novel molecular connector system is used, in which an artificial molecular wire, which is assembled on the gold surface, was plugged into PSI by reconstitution. Analy...

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Published in:Angewandte Chemie (International ed.) 2009-02, Vol.48 (9), p.1585-1587
Main Authors: Terasaki, Nao, Yamamoto, Noritaka, Hiraga, Takashi, Yamanoi, Yoshinori, Yonezawa, Tetsu, Nishihara, Hiroshi, Ohmori, Tsutomu, Sakai, Makoto, Fujii, Masaaki, Tohri, Akihiko, Iwai, Masako, Inoue, Yasunori, Yoneyama, Satoshi, Minakata, Makoto, Enami, Isao
Format: Article
Language:English
Subjects:
biocomponents
Electrodes
electron transfer
Electron Transport
Gold - chemistry
Kinetics
Metal Nanoparticles - chemistry
molecular electronics
photocurrent
photosynthesis
Photosystem I Protein Complex - chemistry
Photosystem I Protein Complex - metabolism
Vitamin K 1 - chemistry
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container_title Angewandte Chemie (International ed.)
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creator Terasaki, Nao
Yamamoto, Noritaka
Hiraga, Takashi
Yamanoi, Yoshinori
Yonezawa, Tetsu
Nishihara, Hiroshi
Ohmori, Tsutomu
Sakai, Makoto
Fujii, Masaaki
Tohri, Akihiko
Iwai, Masako
Inoue, Yasunori
Yoneyama, Satoshi
Minakata, Makoto
Enami, Isao
description Plug and play: Photoinduced electron transfer occurs from photoexcited P700 in photosystem I (PSI) to a gold surface (see picture). A novel molecular connector system is used, in which an artificial molecular wire, which is assembled on the gold surface, was plugged into PSI by reconstitution. Analysis of the photoelectron transfer kinetics proved both the output of electrons from PSI and the effectiveness of the molecular wire.
doi_str_mv 10.1002/anie.200805748
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source Wiley
subjects biocomponents
Electrodes
electron transfer
Electron Transport
Gold - chemistry
Kinetics
Metal Nanoparticles - chemistry
molecular electronics
photocurrent
photosynthesis
Photosystem I Protein Complex - chemistry
Photosystem I Protein Complex - metabolism
Vitamin K 1 - chemistry
title Plugging a Molecular Wire into Photosystem I: Reconstitution of the Photoelectric Conversion System on a Gold Electrode
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