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Wavelength‐Tunable Mid‐Infrared Lasing from Black Phosphorus Nanosheets

Van der Waals layered semiconductor materials own unique physical properties and have attracted intense interest in developing high‐performance electronic and photonic devices. Among them, black phosphorus (BP) is distinct for its layer number‐tuned direct band gap which spans from near‐ to mid‐infr...

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Published in:Advanced materials (Weinheim) 2020-04, Vol.32 (17), p.e1808319-n/a
Main Authors: Zhang, Yushuang, Wang, Shaowei, Chen, Shula, Zhang, Qinglin, Wang, Xiao, Zhu, Xiaoli, Zhang, Xuehong, Xu, Xing, Yang, Tiefeng, He, Mai, Yang, Xin, Li, Ziwei, Chen, Xu, Wu, Mingfei, Lu, Yuerui, Ma, Renmin, Lu, Wei, Pan, Anlian
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cited_by cdi_FETCH-LOGICAL-c3739-1cf74eb18e60ee072e9aef12de4f21f27b7bdcf49438333e18ce48482bb19bdb3
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creator Zhang, Yushuang
Wang, Shaowei
Chen, Shula
Zhang, Qinglin
Wang, Xiao
Zhu, Xiaoli
Zhang, Xuehong
Xu, Xing
Yang, Tiefeng
He, Mai
Yang, Xin
Li, Ziwei
Chen, Xu
Wu, Mingfei
Lu, Yuerui
Ma, Renmin
Lu, Wei
Pan, Anlian
description Van der Waals layered semiconductor materials own unique physical properties and have attracted intense interest in developing high‐performance electronic and photonic devices. Among them, black phosphorus (BP) is distinct for its layer number‐tuned direct band gap which spans from near‐ to mid‐infrared (MIR) waveband. In addition, the puckered honey comb crystal lattice endows the material with highly linear‐polarized emission and marked anisotropy in carrier transportation. These unique material properties render BP as an intriguing and promising building block for constructing mid‐infrared‐ranged coherent light sources. Here, a room temperature surface‐emitting MIR laser based on single crystalline BP nanosheets coupled with a distributed Bragg reflector cavity is reported. MIR stimulated emission at 3611 nm is achieved with a near‐unity linear polarization, which exhibits robust thermal stability up to 360 K. Most importantly, the lasing wavelength can be tuned from 3425 to 4068 nm by varying the cavity length via thickness control of BP layer. The demonstrated highly polarized lasing output and wavelength‐tunable capacity of the proposed device scheme in MIR spectral range opens up promising opportunities for a broad array of applications in polarization‐resolved IR imaging, range‐finding, and free space quantum communications. A vertical surface‐emitting wavelength‐tunable mid‐infrared lasing is achieved from black phosphorus nanosheets embedded in distributed Bragg reflector microcavities.
doi_str_mv 10.1002/adma.201808319
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Among them, black phosphorus (BP) is distinct for its layer number‐tuned direct band gap which spans from near‐ to mid‐infrared (MIR) waveband. In addition, the puckered honey comb crystal lattice endows the material with highly linear‐polarized emission and marked anisotropy in carrier transportation. These unique material properties render BP as an intriguing and promising building block for constructing mid‐infrared‐ranged coherent light sources. Here, a room temperature surface‐emitting MIR laser based on single crystalline BP nanosheets coupled with a distributed Bragg reflector cavity is reported. MIR stimulated emission at 3611 nm is achieved with a near‐unity linear polarization, which exhibits robust thermal stability up to 360 K. Most importantly, the lasing wavelength can be tuned from 3425 to 4068 nm by varying the cavity length via thickness control of BP layer. The demonstrated highly polarized lasing output and wavelength‐tunable capacity of the proposed device scheme in MIR spectral range opens up promising opportunities for a broad array of applications in polarization‐resolved IR imaging, range‐finding, and free space quantum communications. 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The demonstrated highly polarized lasing output and wavelength‐tunable capacity of the proposed device scheme in MIR spectral range opens up promising opportunities for a broad array of applications in polarization‐resolved IR imaging, range‐finding, and free space quantum communications. 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The demonstrated highly polarized lasing output and wavelength‐tunable capacity of the proposed device scheme in MIR spectral range opens up promising opportunities for a broad array of applications in polarization‐resolved IR imaging, range‐finding, and free space quantum communications. A vertical surface‐emitting wavelength‐tunable mid‐infrared lasing is achieved from black phosphorus nanosheets embedded in distributed Bragg reflector microcavities.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>32159904</pmid><doi>10.1002/adma.201808319</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-3335-3067</orcidid></addata></record>
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subjects Anisotropy
black phosphorus
Coherent light
Crystal lattices
Electronic devices
Emission
Infrared imaging
Laser applications
Lasing
Light sources
Linear polarization
Material properties
Materials science
mid‐infrared lasing
Nanosheets
Phosphorus
Physical properties
Room temperature
Semiconductor materials
Stimulated emission
Thermal stability
Thickness
title Wavelength‐Tunable Mid‐Infrared Lasing from Black Phosphorus Nanosheets
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