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Groundwater contamination with volatile organic compounds in urban and industrial areas: analysis of co-occurrence and land use effects
Chlorinated solvents and trihalomethanes were the most frequently detected volatile organic compound (VOC) groups in groundwater in two metropolitan cities and three industrial complexes in Korea. Groundwater contamination with carbon tetrachloride and chloroform was noticeable in the industrial com...
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Published in: | Environmental earth sciences 2015-08, Vol.74 (4), p.3661-3677 |
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description | Chlorinated solvents and trihalomethanes were the most frequently detected volatile organic compound (VOC) groups in groundwater in two metropolitan cities and three industrial complexes in Korea. Groundwater contamination with carbon tetrachloride and chloroform was noticeable in the industrial complexes, while MTBE was frequently detected only in metropolitan cities. In particular, groundwater was severely contaminated with chlorinated solvents and their dechlorination intermediates, including cis-1,2-DCE from TCE and 1,1-DCE from 1,1,1-TCA. Their co-occurrences were analyzed based on detection frequencies, rates of exceeding the water quality criteria, and a correlation matrix. Meanwhile, frequently co-occurring VOCs and VOC concentrations exceeding the water quality criteria were detected in only a few samples, which demonstrates the effects of land use due to the application of various types of VOCs. Thus, the effects of local land use were investigated by categorizing groundwater samples based on land use at the sampling locations; the effects of regional land use were assessed using factor analysis with administrative district statistics. The assessment results showed that public garages at the sampling locations were correlated with groundwater contamination. The detection of MTBE was correlated with vehicle use, while the detection of both toluene and chloroform was correlated with manufacturing and sewage collection and disposal systems; PCE was correlated with hazardous wastes. The contribution of this work is that the co-occurrence of some VOCs and persistent dechlorination intermediates was analyzed using a correlation matrix. Local and regional land uses were separately defined; their impacts on groundwater quality were assessed. Furthermore, a factor analysis included anthropogenic variables and VOC detection rates to better define latent variables. |
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Groundwater contamination with carbon tetrachloride and chloroform was noticeable in the industrial complexes, while MTBE was frequently detected only in metropolitan cities. In particular, groundwater was severely contaminated with chlorinated solvents and their dechlorination intermediates, including cis-1,2-DCE from TCE and 1,1-DCE from 1,1,1-TCA. Their co-occurrences were analyzed based on detection frequencies, rates of exceeding the water quality criteria, and a correlation matrix. Meanwhile, frequently co-occurring VOCs and VOC concentrations exceeding the water quality criteria were detected in only a few samples, which demonstrates the effects of land use due to the application of various types of VOCs. Thus, the effects of local land use were investigated by categorizing groundwater samples based on land use at the sampling locations; the effects of regional land use were assessed using factor analysis with administrative district statistics. The assessment results showed that public garages at the sampling locations were correlated with groundwater contamination. The detection of MTBE was correlated with vehicle use, while the detection of both toluene and chloroform was correlated with manufacturing and sewage collection and disposal systems; PCE was correlated with hazardous wastes. The contribution of this work is that the co-occurrence of some VOCs and persistent dechlorination intermediates was analyzed using a correlation matrix. Local and regional land uses were separately defined; their impacts on groundwater quality were assessed. Furthermore, a factor analysis included anthropogenic variables and VOC detection rates to better define latent variables.</description><identifier>ISSN: 1866-6280</identifier><identifier>EISSN: 1866-6299</identifier><identifier>DOI: 10.1007/s12665-015-4551-z</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Biogeosciences ; carbon tetrachloride ; chloroform ; cities ; dechlorination ; Earth and Environmental Science ; Earth Sciences ; Environmental impact ; Environmental Science and Engineering ; factor analysis ; Geochemistry ; Geology ; groundwater ; groundwater contamination ; Groundwater pollution ; Hydrology/Water Resources ; Land use ; manufacturing ; Original Article ; sampling ; sewage ; solvents ; Terrestrial Pollution ; toluene ; VOCs ; Volatile organic compounds ; water quality ; water quality criteria</subject><ispartof>Environmental earth sciences, 2015-08, Vol.74 (4), p.3661-3677</ispartof><rights>Springer-Verlag Berlin Heidelberg 2015</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a466t-98a0de7b73bda3fc14e2b2cee0f9142df696582f365900234d779d8e6de1fe103</citedby><cites>FETCH-LOGICAL-a466t-98a0de7b73bda3fc14e2b2cee0f9142df696582f365900234d779d8e6de1fe103</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,786,790,27957,27958</link.rule.ids></links><search><creatorcontrib>Yu, Soonyoung</creatorcontrib><creatorcontrib>Lee, Pyeong-Koo</creatorcontrib><creatorcontrib>Hwang, Sang-Il</creatorcontrib><title>Groundwater contamination with volatile organic compounds in urban and industrial areas: analysis of co-occurrence and land use effects</title><title>Environmental earth sciences</title><addtitle>Environ Earth Sci</addtitle><description>Chlorinated solvents and trihalomethanes were the most frequently detected volatile organic compound (VOC) groups in groundwater in two metropolitan cities and three industrial complexes in Korea. Groundwater contamination with carbon tetrachloride and chloroform was noticeable in the industrial complexes, while MTBE was frequently detected only in metropolitan cities. In particular, groundwater was severely contaminated with chlorinated solvents and their dechlorination intermediates, including cis-1,2-DCE from TCE and 1,1-DCE from 1,1,1-TCA. Their co-occurrences were analyzed based on detection frequencies, rates of exceeding the water quality criteria, and a correlation matrix. Meanwhile, frequently co-occurring VOCs and VOC concentrations exceeding the water quality criteria were detected in only a few samples, which demonstrates the effects of land use due to the application of various types of VOCs. Thus, the effects of local land use were investigated by categorizing groundwater samples based on land use at the sampling locations; the effects of regional land use were assessed using factor analysis with administrative district statistics. The assessment results showed that public garages at the sampling locations were correlated with groundwater contamination. The detection of MTBE was correlated with vehicle use, while the detection of both toluene and chloroform was correlated with manufacturing and sewage collection and disposal systems; PCE was correlated with hazardous wastes. The contribution of this work is that the co-occurrence of some VOCs and persistent dechlorination intermediates was analyzed using a correlation matrix. Local and regional land uses were separately defined; their impacts on groundwater quality were assessed. Furthermore, a factor analysis included anthropogenic variables and VOC detection rates to better define latent variables.</description><subject>Biogeosciences</subject><subject>carbon tetrachloride</subject><subject>chloroform</subject><subject>cities</subject><subject>dechlorination</subject><subject>Earth and Environmental Science</subject><subject>Earth Sciences</subject><subject>Environmental impact</subject><subject>Environmental Science and Engineering</subject><subject>factor analysis</subject><subject>Geochemistry</subject><subject>Geology</subject><subject>groundwater</subject><subject>groundwater contamination</subject><subject>Groundwater pollution</subject><subject>Hydrology/Water Resources</subject><subject>Land use</subject><subject>manufacturing</subject><subject>Original Article</subject><subject>sampling</subject><subject>sewage</subject><subject>solvents</subject><subject>Terrestrial Pollution</subject><subject>toluene</subject><subject>VOCs</subject><subject>Volatile organic compounds</subject><subject>water quality</subject><subject>water quality criteria</subject><issn>1866-6280</issn><issn>1866-6299</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNp9kc9qFTEUhwexYGn7AK4MuHEzNieZSTLupNg_UHBhuw65mZNrytzkmjNjaV_A1zbXEREXZpHkhO875PBrmtfA3wPn-pxAKNW3HPq263ton180x2CUapUYhpd_7oa_as6IHnhdEuTA1XHz46rkJY2PbsbCfE6z28Xk5pgTe4zzV_Y9T7WakOWydSn6yuz2B4NYTGwpG5eYS2MtxoXmEt3EXEFHH-qrm54oEsuhSm32fikFk8df_HTYFkKGIaCf6bQ5Cm4iPPt9njT3l5_uLq7b289XNxcfb1vXKTW3g3F8RL3RcjM6GTx0KDbCI_IwQCfGoAbVGxGk6gfOhexGrYfRoBoRAgKXJ827te--5G8L0mx3kTxO9T-YF7JguJFacugq-vYf9CEvpU5VKa2FBKMBKgUr5UsmKhjsvsSdK08WuD2kY9d0bE3HHtKxz9URq0OVTVssf3X-j_RmlYLL1m1LJHv_RVSgzglSGiN_AsXengg</recordid><startdate>20150801</startdate><enddate>20150801</enddate><creator>Yu, Soonyoung</creator><creator>Lee, Pyeong-Koo</creator><creator>Hwang, Sang-Il</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>FBQ</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7ST</scope><scope>7TG</scope><scope>7UA</scope><scope>7XB</scope><scope>88I</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>F1W</scope><scope>GNUQQ</scope><scope>H96</scope><scope>HCIFZ</scope><scope>KL.</scope><scope>L.G</scope><scope>M2P</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>SOI</scope><scope>7QH</scope><scope>7TV</scope><scope>H97</scope></search><sort><creationdate>20150801</creationdate><title>Groundwater contamination with volatile organic compounds in urban and industrial areas: analysis of co-occurrence and land use effects</title><author>Yu, Soonyoung ; Lee, Pyeong-Koo ; Hwang, Sang-Il</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a466t-98a0de7b73bda3fc14e2b2cee0f9142df696582f365900234d779d8e6de1fe103</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Biogeosciences</topic><topic>carbon tetrachloride</topic><topic>chloroform</topic><topic>cities</topic><topic>dechlorination</topic><topic>Earth and Environmental Science</topic><topic>Earth Sciences</topic><topic>Environmental impact</topic><topic>Environmental Science and Engineering</topic><topic>factor analysis</topic><topic>Geochemistry</topic><topic>Geology</topic><topic>groundwater</topic><topic>groundwater contamination</topic><topic>Groundwater pollution</topic><topic>Hydrology/Water Resources</topic><topic>Land use</topic><topic>manufacturing</topic><topic>Original Article</topic><topic>sampling</topic><topic>sewage</topic><topic>solvents</topic><topic>Terrestrial Pollution</topic><topic>toluene</topic><topic>VOCs</topic><topic>Volatile organic compounds</topic><topic>water quality</topic><topic>water quality criteria</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yu, Soonyoung</creatorcontrib><creatorcontrib>Lee, Pyeong-Koo</creatorcontrib><creatorcontrib>Hwang, Sang-Il</creatorcontrib><collection>AGRIS</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Water Resources Abstracts</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Natural Science Collection</collection><collection>Earth, Atmospheric & Aquatic Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>ProQuest Central Student</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>SciTech Premium Collection</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Science Database</collection><collection>Environmental Science Database</collection><collection>Earth, Atmospheric & Aquatic Science Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>Environment Abstracts</collection><collection>Aqualine</collection><collection>Pollution Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><jtitle>Environmental earth sciences</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yu, Soonyoung</au><au>Lee, Pyeong-Koo</au><au>Hwang, Sang-Il</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Groundwater contamination with volatile organic compounds in urban and industrial areas: analysis of co-occurrence and land use effects</atitle><jtitle>Environmental earth sciences</jtitle><stitle>Environ Earth Sci</stitle><date>2015-08-01</date><risdate>2015</risdate><volume>74</volume><issue>4</issue><spage>3661</spage><epage>3677</epage><pages>3661-3677</pages><issn>1866-6280</issn><eissn>1866-6299</eissn><notes>http://dx.doi.org/10.1007/s12665-015-4551-z</notes><notes>ObjectType-Article-1</notes><notes>SourceType-Scholarly Journals-1</notes><notes>ObjectType-Feature-2</notes><notes>content type line 23</notes><abstract>Chlorinated solvents and trihalomethanes were the most frequently detected volatile organic compound (VOC) groups in groundwater in two metropolitan cities and three industrial complexes in Korea. Groundwater contamination with carbon tetrachloride and chloroform was noticeable in the industrial complexes, while MTBE was frequently detected only in metropolitan cities. In particular, groundwater was severely contaminated with chlorinated solvents and their dechlorination intermediates, including cis-1,2-DCE from TCE and 1,1-DCE from 1,1,1-TCA. Their co-occurrences were analyzed based on detection frequencies, rates of exceeding the water quality criteria, and a correlation matrix. Meanwhile, frequently co-occurring VOCs and VOC concentrations exceeding the water quality criteria were detected in only a few samples, which demonstrates the effects of land use due to the application of various types of VOCs. Thus, the effects of local land use were investigated by categorizing groundwater samples based on land use at the sampling locations; the effects of regional land use were assessed using factor analysis with administrative district statistics. The assessment results showed that public garages at the sampling locations were correlated with groundwater contamination. The detection of MTBE was correlated with vehicle use, while the detection of both toluene and chloroform was correlated with manufacturing and sewage collection and disposal systems; PCE was correlated with hazardous wastes. The contribution of this work is that the co-occurrence of some VOCs and persistent dechlorination intermediates was analyzed using a correlation matrix. Local and regional land uses were separately defined; their impacts on groundwater quality were assessed. Furthermore, a factor analysis included anthropogenic variables and VOC detection rates to better define latent variables.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s12665-015-4551-z</doi><tpages>17</tpages></addata></record> |
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subjects | Biogeosciences carbon tetrachloride chloroform cities dechlorination Earth and Environmental Science Earth Sciences Environmental impact Environmental Science and Engineering factor analysis Geochemistry Geology groundwater groundwater contamination Groundwater pollution Hydrology/Water Resources Land use manufacturing Original Article sampling sewage solvents Terrestrial Pollution toluene VOCs Volatile organic compounds water quality water quality criteria |
title | Groundwater contamination with volatile organic compounds in urban and industrial areas: analysis of co-occurrence and land use effects |
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