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Enhanced moisture stability of MAPbI3 perovskite solar cells through Barium doping
[Display omitted] •We have fabricated pristine and various concentration Ba doped perovskite solar cells (PSCs) through an intense pulsed light (IPL) process.•The XRD analysis has confirmed the formation of pristine and Ba doped perovskite films.•After systematic photovoltaic analysis, it was found...
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| Published in: | Solar energy 2019-09, Vol.190, p.396-404 |
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| cited_by | cdi_FETCH-LOGICAL-c291t-a1c5c7916acf522a04d68d03bd678e833dbf8d994b56a2b954808d64295afd803 |
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| cites | cdi_FETCH-LOGICAL-c291t-a1c5c7916acf522a04d68d03bd678e833dbf8d994b56a2b954808d64295afd803 |
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| container_title | Solar energy |
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| creator | Bahadur, Jitendra Ghahremani, Amir H. Gupta, Sunil Druffel, Thad Sunkara, Mahendra K. Pal, Kaushik |
| description | [Display omitted]
•We have fabricated pristine and various concentration Ba doped perovskite solar cells (PSCs) through an intense pulsed light (IPL) process.•The XRD analysis has confirmed the formation of pristine and Ba doped perovskite films.•After systematic photovoltaic analysis, it was found that 2.0 mol% exhibited long-term stability in comparison to pristine PSC.
Rapid growth within performance and stability of organic-inorganic halide-based perovskite solar cells (PSCs) has made this emerging photovoltaics a great potential for further research towards successful commercialization. However, two major issues of: (i) Structural ambient stability, and (ii) Toxicity, caused by the presence of Pb content, are the pivotal obstacles for the commercialization of environmental friendly PSC. In this regard, we are introducing a highly ambient stable PSC through the incorporation of barium (Ba) with successful ultrashort annealing through intense pulsed light (IPL). The ambient stability of Ba doped perovskite thin films was explored in the humidity range of 35–68%. The power conversion efficiency (PCE) of fabricated devices were found to be 8.99, 7.39, 6.94, 6.60, 5.98 and 3.82% for pristine, 1, 2, 5, 10, and 20 mol% Ba doping, respectively. Afterwards, fabricated devices were kept in ambient environment under dark for 20 days. With systematic photovoltaic analysis, it was observed that the 2.0 mol% Ba doped PSC exhibited 8.0% efficiency drop (from 6.94 to 6.38%), whereas the PCE of pristine based devices decreased from 8.99 to 2.60%, demonstrating an almost 71.0% drop. Our photovoltaic results demonstrated a great improvement within the ambient stability of PSC without any encapsulation which can indicate Ba doping as highly promising approach for the fabrication of PSC with higher ambient stability. |
| doi_str_mv | 10.1016/j.solener.2019.08.033 |
| format | article |
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•We have fabricated pristine and various concentration Ba doped perovskite solar cells (PSCs) through an intense pulsed light (IPL) process.•The XRD analysis has confirmed the formation of pristine and Ba doped perovskite films.•After systematic photovoltaic analysis, it was found that 2.0 mol% exhibited long-term stability in comparison to pristine PSC.
Rapid growth within performance and stability of organic-inorganic halide-based perovskite solar cells (PSCs) has made this emerging photovoltaics a great potential for further research towards successful commercialization. However, two major issues of: (i) Structural ambient stability, and (ii) Toxicity, caused by the presence of Pb content, are the pivotal obstacles for the commercialization of environmental friendly PSC. In this regard, we are introducing a highly ambient stable PSC through the incorporation of barium (Ba) with successful ultrashort annealing through intense pulsed light (IPL). The ambient stability of Ba doped perovskite thin films was explored in the humidity range of 35–68%. The power conversion efficiency (PCE) of fabricated devices were found to be 8.99, 7.39, 6.94, 6.60, 5.98 and 3.82% for pristine, 1, 2, 5, 10, and 20 mol% Ba doping, respectively. Afterwards, fabricated devices were kept in ambient environment under dark for 20 days. With systematic photovoltaic analysis, it was observed that the 2.0 mol% Ba doped PSC exhibited 8.0% efficiency drop (from 6.94 to 6.38%), whereas the PCE of pristine based devices decreased from 8.99 to 2.60%, demonstrating an almost 71.0% drop. Our photovoltaic results demonstrated a great improvement within the ambient stability of PSC without any encapsulation which can indicate Ba doping as highly promising approach for the fabrication of PSC with higher ambient stability.</description><identifier>ISSN: 0038-092X</identifier><identifier>EISSN: 1471-1257</identifier><identifier>DOI: 10.1016/j.solener.2019.08.033</identifier><language>eng</language><publisher>New York: Elsevier Ltd</publisher><subject>Barium ; Barium doping ; Commercialization ; Doping ; Energy conversion efficiency ; Fabrication ; Intense pulsed laser ; Lead ; Perovskite solar cells ; Perovskites ; Photovoltaic cells ; Photovoltaics ; Solar cells ; Solar energy ; Stability ; Structural stability ; Thin films ; Toxicity</subject><ispartof>Solar energy, 2019-09, Vol.190, p.396-404</ispartof><rights>2019 International Solar Energy Society</rights><rights>Copyright Pergamon Press Inc. Sep 15, 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c291t-a1c5c7916acf522a04d68d03bd678e833dbf8d994b56a2b954808d64295afd803</citedby><cites>FETCH-LOGICAL-c291t-a1c5c7916acf522a04d68d03bd678e833dbf8d994b56a2b954808d64295afd803</cites><orcidid>0000-0002-7409-9344</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,783,787,27938,27939</link.rule.ids></links><search><creatorcontrib>Bahadur, Jitendra</creatorcontrib><creatorcontrib>Ghahremani, Amir H.</creatorcontrib><creatorcontrib>Gupta, Sunil</creatorcontrib><creatorcontrib>Druffel, Thad</creatorcontrib><creatorcontrib>Sunkara, Mahendra K.</creatorcontrib><creatorcontrib>Pal, Kaushik</creatorcontrib><title>Enhanced moisture stability of MAPbI3 perovskite solar cells through Barium doping</title><title>Solar energy</title><description>[Display omitted]
•We have fabricated pristine and various concentration Ba doped perovskite solar cells (PSCs) through an intense pulsed light (IPL) process.•The XRD analysis has confirmed the formation of pristine and Ba doped perovskite films.•After systematic photovoltaic analysis, it was found that 2.0 mol% exhibited long-term stability in comparison to pristine PSC.
Rapid growth within performance and stability of organic-inorganic halide-based perovskite solar cells (PSCs) has made this emerging photovoltaics a great potential for further research towards successful commercialization. However, two major issues of: (i) Structural ambient stability, and (ii) Toxicity, caused by the presence of Pb content, are the pivotal obstacles for the commercialization of environmental friendly PSC. In this regard, we are introducing a highly ambient stable PSC through the incorporation of barium (Ba) with successful ultrashort annealing through intense pulsed light (IPL). The ambient stability of Ba doped perovskite thin films was explored in the humidity range of 35–68%. The power conversion efficiency (PCE) of fabricated devices were found to be 8.99, 7.39, 6.94, 6.60, 5.98 and 3.82% for pristine, 1, 2, 5, 10, and 20 mol% Ba doping, respectively. Afterwards, fabricated devices were kept in ambient environment under dark for 20 days. With systematic photovoltaic analysis, it was observed that the 2.0 mol% Ba doped PSC exhibited 8.0% efficiency drop (from 6.94 to 6.38%), whereas the PCE of pristine based devices decreased from 8.99 to 2.60%, demonstrating an almost 71.0% drop. Our photovoltaic results demonstrated a great improvement within the ambient stability of PSC without any encapsulation which can indicate Ba doping as highly promising approach for the fabrication of PSC with higher ambient stability.</description><subject>Barium</subject><subject>Barium doping</subject><subject>Commercialization</subject><subject>Doping</subject><subject>Energy conversion efficiency</subject><subject>Fabrication</subject><subject>Intense pulsed laser</subject><subject>Lead</subject><subject>Perovskite solar cells</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>Photovoltaics</subject><subject>Solar cells</subject><subject>Solar energy</subject><subject>Stability</subject><subject>Structural stability</subject><subject>Thin films</subject><subject>Toxicity</subject><issn>0038-092X</issn><issn>1471-1257</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqFkE1LwzAYx4MoOKcfQQh4bn2SNm1ykjmmDiaKKHgLaZJumV0zk3awb2_Hdvf0HP5vPD-EbgmkBEhxv06jb2xrQ0qBiBR4Cll2hkYkL0lCKCvP0Qgg4wkI-n2JrmJcA5CS8HKEPmbtSrXaGrzxLnZ9sDh2qnKN6_bY1_h18l7NM7y1we_ij-sG2TcqYG2bJuJuFXy_XOFHFVy_wcZvXbu8Rhe1aqK9Od0x-nqafU5fksXb83w6WSSaCtIlimimS0EKpWtGqYLcFNxAVpmi5JZnmalqboTIK1YoWgmWc-CmyKlgqjYcsjG6O_Zug__tbezk2vehHSYlpYKXBWXABhc7unTwMQZby21wGxX2koA84JNrecInD_gkcDngG3IPx5wdXti5QY3a2QMpF6zupPHun4Y__aZ7xw</recordid><startdate>20190915</startdate><enddate>20190915</enddate><creator>Bahadur, Jitendra</creator><creator>Ghahremani, Amir H.</creator><creator>Gupta, Sunil</creator><creator>Druffel, Thad</creator><creator>Sunkara, Mahendra K.</creator><creator>Pal, Kaushik</creator><general>Elsevier Ltd</general><general>Pergamon Press Inc</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7ST</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope><scope>L7M</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0002-7409-9344</orcidid></search><sort><creationdate>20190915</creationdate><title>Enhanced moisture stability of MAPbI3 perovskite solar cells through Barium doping</title><author>Bahadur, Jitendra ; Ghahremani, Amir H. ; Gupta, Sunil ; Druffel, Thad ; Sunkara, Mahendra K. ; Pal, Kaushik</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c291t-a1c5c7916acf522a04d68d03bd678e833dbf8d994b56a2b954808d64295afd803</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Barium</topic><topic>Barium doping</topic><topic>Commercialization</topic><topic>Doping</topic><topic>Energy conversion efficiency</topic><topic>Fabrication</topic><topic>Intense pulsed laser</topic><topic>Lead</topic><topic>Perovskite solar cells</topic><topic>Perovskites</topic><topic>Photovoltaic cells</topic><topic>Photovoltaics</topic><topic>Solar cells</topic><topic>Solar energy</topic><topic>Stability</topic><topic>Structural stability</topic><topic>Thin films</topic><topic>Toxicity</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bahadur, Jitendra</creatorcontrib><creatorcontrib>Ghahremani, Amir H.</creatorcontrib><creatorcontrib>Gupta, Sunil</creatorcontrib><creatorcontrib>Druffel, Thad</creatorcontrib><creatorcontrib>Sunkara, Mahendra K.</creatorcontrib><creatorcontrib>Pal, Kaushik</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Environment Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Solar energy</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bahadur, Jitendra</au><au>Ghahremani, Amir H.</au><au>Gupta, Sunil</au><au>Druffel, Thad</au><au>Sunkara, Mahendra K.</au><au>Pal, Kaushik</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced moisture stability of MAPbI3 perovskite solar cells through Barium doping</atitle><jtitle>Solar energy</jtitle><date>2019-09-15</date><risdate>2019</risdate><volume>190</volume><spage>396</spage><epage>404</epage><pages>396-404</pages><issn>0038-092X</issn><eissn>1471-1257</eissn><abstract>[Display omitted]
•We have fabricated pristine and various concentration Ba doped perovskite solar cells (PSCs) through an intense pulsed light (IPL) process.•The XRD analysis has confirmed the formation of pristine and Ba doped perovskite films.•After systematic photovoltaic analysis, it was found that 2.0 mol% exhibited long-term stability in comparison to pristine PSC.
Rapid growth within performance and stability of organic-inorganic halide-based perovskite solar cells (PSCs) has made this emerging photovoltaics a great potential for further research towards successful commercialization. However, two major issues of: (i) Structural ambient stability, and (ii) Toxicity, caused by the presence of Pb content, are the pivotal obstacles for the commercialization of environmental friendly PSC. In this regard, we are introducing a highly ambient stable PSC through the incorporation of barium (Ba) with successful ultrashort annealing through intense pulsed light (IPL). The ambient stability of Ba doped perovskite thin films was explored in the humidity range of 35–68%. The power conversion efficiency (PCE) of fabricated devices were found to be 8.99, 7.39, 6.94, 6.60, 5.98 and 3.82% for pristine, 1, 2, 5, 10, and 20 mol% Ba doping, respectively. Afterwards, fabricated devices were kept in ambient environment under dark for 20 days. With systematic photovoltaic analysis, it was observed that the 2.0 mol% Ba doped PSC exhibited 8.0% efficiency drop (from 6.94 to 6.38%), whereas the PCE of pristine based devices decreased from 8.99 to 2.60%, demonstrating an almost 71.0% drop. Our photovoltaic results demonstrated a great improvement within the ambient stability of PSC without any encapsulation which can indicate Ba doping as highly promising approach for the fabrication of PSC with higher ambient stability.</abstract><cop>New York</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.solener.2019.08.033</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0002-7409-9344</orcidid></addata></record> |
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| subjects | Barium Barium doping Commercialization Doping Energy conversion efficiency Fabrication Intense pulsed laser Lead Perovskite solar cells Perovskites Photovoltaic cells Photovoltaics Solar cells Solar energy Stability Structural stability Thin films Toxicity |
| title | Enhanced moisture stability of MAPbI3 perovskite solar cells through Barium doping |
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