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Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications

•Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity (

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Published in:Journal of alloys and compounds 2021-08, Vol.872, p.159728, Article 159728
Main Authors: Haydoura, M., Benzerga, R., Le Paven, C., Le Gendre, L., Laur, V., Chevalier, A., Sharaiha, A., Tessier, F., Cheviré, F.
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creator Haydoura, M.
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Cheviré, F.
description •Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity (
doi_str_mv 10.1016/j.jallcom.2021.159728
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[Display omitted] In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x&lt;1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. 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[Display omitted] In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x&lt;1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. These features confirm the potential of the paraelectric STLTO compositions in compact antennas radiating at frequencies below 6 GHz.</description><subject>Ceramic powders</subject><subject>Ceramics</subject><subject>Chemical composition</subject><subject>Chemical Sciences</subject><subject>Dielectric loss</subject><subject>Dielectric properties</subject><subject>Dielectric resonator antenna</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>High temperature</subject><subject>Material chemistry</subject><subject>Permittivity</subject><subject>Perovskite materials</subject><subject>Perovskites</subject><subject>Radio antennas</subject><subject>Resonant frequencies</subject><subject>Resonators</subject><subject>Room temperature</subject><subject>Sintering (powder metallurgy)</subject><subject>Solid solutions</subject><issn>0925-8388</issn><issn>1873-4669</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNqFkcFu1DAQhi0EEkvhEZAicWkPWTx2HDtcUFVRirRSkVjO1sSZqA7ZeLHdVcuFK2cekSchSyrEjcuMNPPNr5n5GXsJfA0c6tfDesBxdGG3FlzAGlSjhXnEVmC0LKu6bh6zFW-EKo005il7ltLAOYdGwop9_0gxHNIXn6k4_RTFFsW1PgPOf_34eXe6QbH1x8Jd4Sjizrv0priMYVd0nkZyOXpXuBuM6DJF_w2zD1ORw7_tSClMmEMscMo0TVjgfj9694dNz9mTHsdELx7yCft8-W57cVVurt9_uDjflK4Ck0uaI_VAimPXtqREx01XCWjb3lTaGKEBeyewrVzl2kq3ope1MD3UoDWXUp6ws0X3Bke7j36H8d4G9PbqfGOPNS4FSNGoA8zsq4Xdx_D1llK2Q7iN07yeFUpqUFKJZqbUQrkYUorU_5UFbo--2ME--GKPvtjFl3nu7TJH87kHT9Em52ly1Pk4v8x2wf9H4TcH4JmD</recordid><startdate>20210815</startdate><enddate>20210815</enddate><creator>Haydoura, M.</creator><creator>Benzerga, R.</creator><creator>Le Paven, C.</creator><creator>Le Gendre, L.</creator><creator>Laur, V.</creator><creator>Chevalier, A.</creator><creator>Sharaiha, A.</creator><creator>Tessier, F.</creator><creator>Cheviré, F.</creator><general>Elsevier B.V</general><general>Elsevier BV</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-5755-0041</orcidid><orcidid>https://orcid.org/0000-0002-2017-5233</orcidid><orcidid>https://orcid.org/0000-0001-8078-9301</orcidid><orcidid>https://orcid.org/0000-0002-5605-6113</orcidid><orcidid>https://orcid.org/0000-0002-1253-7011</orcidid></search><sort><creationdate>20210815</creationdate><title>Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications</title><author>Haydoura, M. ; 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[Display omitted] In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x&lt;1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. These features confirm the potential of the paraelectric STLTO compositions in compact antennas radiating at frequencies below 6 GHz.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jallcom.2021.159728</doi><orcidid>https://orcid.org/0000-0002-5755-0041</orcidid><orcidid>https://orcid.org/0000-0002-2017-5233</orcidid><orcidid>https://orcid.org/0000-0001-8078-9301</orcidid><orcidid>https://orcid.org/0000-0002-5605-6113</orcidid><orcidid>https://orcid.org/0000-0002-1253-7011</orcidid><oa>free_for_read</oa></addata></record>
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ispartof Journal of alloys and compounds, 2021-08, Vol.872, p.159728, Article 159728
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1873-4669
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subjects Ceramic powders
Ceramics
Chemical composition
Chemical Sciences
Dielectric loss
Dielectric properties
Dielectric resonator antenna
Ferroelectric materials
Ferroelectricity
High temperature
Material chemistry
Permittivity
Perovskite materials
Perovskites
Radio antennas
Resonant frequencies
Resonators
Room temperature
Sintering (powder metallurgy)
Solid solutions
title Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications
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