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Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications
•Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity (
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Published in: | Journal of alloys and compounds 2021-08, Vol.872, p.159728, Article 159728 |
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container_title | Journal of alloys and compounds |
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creator | Haydoura, M. Benzerga, R. Le Paven, C. Le Gendre, L. Laur, V. Chevalier, A. Sharaiha, A. Tessier, F. Cheviré, F. |
description | •Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity ( |
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[Display omitted]
In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x<1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. These features confirm the potential of the paraelectric STLTO compositions in compact antennas radiating at frequencies below 6 GHz.</description><identifier>ISSN: 0925-8388</identifier><identifier>EISSN: 1873-4669</identifier><identifier>DOI: 10.1016/j.jallcom.2021.159728</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Ceramic powders ; Ceramics ; Chemical composition ; Chemical Sciences ; Dielectric loss ; Dielectric properties ; Dielectric resonator antenna ; Ferroelectric materials ; Ferroelectricity ; High temperature ; Material chemistry ; Permittivity ; Perovskite materials ; Perovskites ; Radio antennas ; Resonant frequencies ; Resonators ; Room temperature ; Sintering (powder metallurgy) ; Solid solutions</subject><ispartof>Journal of alloys and compounds, 2021-08, Vol.872, p.159728, Article 159728</ispartof><rights>2021 Elsevier B.V.</rights><rights>Copyright Elsevier BV Aug 15, 2021</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c418t-e418ef1e50adbbe52d08d421bbf84788271afc2ab4c4cb47b2f3628f161770333</citedby><cites>FETCH-LOGICAL-c418t-e418ef1e50adbbe52d08d421bbf84788271afc2ab4c4cb47b2f3628f161770333</cites><orcidid>0000-0002-5755-0041 ; 0000-0002-2017-5233 ; 0000-0001-8078-9301 ; 0000-0002-5605-6113 ; 0000-0002-1253-7011</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,315,786,790,891,27957,27958</link.rule.ids><backlink>$$Uhttps://univ-rennes.hal.science/hal-03213295$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Haydoura, M.</creatorcontrib><creatorcontrib>Benzerga, R.</creatorcontrib><creatorcontrib>Le Paven, C.</creatorcontrib><creatorcontrib>Le Gendre, L.</creatorcontrib><creatorcontrib>Laur, V.</creatorcontrib><creatorcontrib>Chevalier, A.</creatorcontrib><creatorcontrib>Sharaiha, A.</creatorcontrib><creatorcontrib>Tessier, F.</creatorcontrib><creatorcontrib>Cheviré, F.</creatorcontrib><title>Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications</title><title>Journal of alloys and compounds</title><description>•Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity (<100) and low dielectric loss (<8 × 10−3) at 2 GHz for x < 1.•Simulation, realization and measurement of a compact dielectric resonator antenna.•Bandwidth of 4.9% and a gain of 6.4 dB are obtained at the frequency of 5.80 GHz.
[Display omitted]
In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x<1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. These features confirm the potential of the paraelectric STLTO compositions in compact antennas radiating at frequencies below 6 GHz.</description><subject>Ceramic powders</subject><subject>Ceramics</subject><subject>Chemical composition</subject><subject>Chemical Sciences</subject><subject>Dielectric loss</subject><subject>Dielectric properties</subject><subject>Dielectric resonator antenna</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>High temperature</subject><subject>Material chemistry</subject><subject>Permittivity</subject><subject>Perovskite materials</subject><subject>Perovskites</subject><subject>Radio antennas</subject><subject>Resonant frequencies</subject><subject>Resonators</subject><subject>Room temperature</subject><subject>Sintering (powder metallurgy)</subject><subject>Solid solutions</subject><issn>0925-8388</issn><issn>1873-4669</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNqFkcFu1DAQhi0EEkvhEZAicWkPWTx2HDtcUFVRirRSkVjO1sSZqA7ZeLHdVcuFK2cekSchSyrEjcuMNPPNr5n5GXsJfA0c6tfDesBxdGG3FlzAGlSjhXnEVmC0LKu6bh6zFW-EKo005il7ltLAOYdGwop9_0gxHNIXn6k4_RTFFsW1PgPOf_34eXe6QbH1x8Jd4Sjizrv0priMYVd0nkZyOXpXuBuM6DJF_w2zD1ORw7_tSClMmEMscMo0TVjgfj9694dNz9mTHsdELx7yCft8-W57cVVurt9_uDjflK4Ck0uaI_VAimPXtqREx01XCWjb3lTaGKEBeyewrVzl2kq3ope1MD3UoDWXUp6ws0X3Bke7j36H8d4G9PbqfGOPNS4FSNGoA8zsq4Xdx_D1llK2Q7iN07yeFUpqUFKJZqbUQrkYUorU_5UFbo--2ME--GKPvtjFl3nu7TJH87kHT9Em52ly1Pk4v8x2wf9H4TcH4JmD</recordid><startdate>20210815</startdate><enddate>20210815</enddate><creator>Haydoura, M.</creator><creator>Benzerga, R.</creator><creator>Le Paven, C.</creator><creator>Le Gendre, L.</creator><creator>Laur, V.</creator><creator>Chevalier, A.</creator><creator>Sharaiha, A.</creator><creator>Tessier, F.</creator><creator>Cheviré, F.</creator><general>Elsevier B.V</general><general>Elsevier BV</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>1XC</scope><scope>VOOES</scope><orcidid>https://orcid.org/0000-0002-5755-0041</orcidid><orcidid>https://orcid.org/0000-0002-2017-5233</orcidid><orcidid>https://orcid.org/0000-0001-8078-9301</orcidid><orcidid>https://orcid.org/0000-0002-5605-6113</orcidid><orcidid>https://orcid.org/0000-0002-1253-7011</orcidid></search><sort><creationdate>20210815</creationdate><title>Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications</title><author>Haydoura, M. ; Benzerga, R. ; Le Paven, C. ; Le Gendre, L. ; Laur, V. ; Chevalier, A. ; Sharaiha, A. ; Tessier, F. ; Cheviré, F.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c418t-e418ef1e50adbbe52d08d421bbf84788271afc2ab4c4cb47b2f3628f161770333</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Ceramic powders</topic><topic>Ceramics</topic><topic>Chemical composition</topic><topic>Chemical Sciences</topic><topic>Dielectric loss</topic><topic>Dielectric properties</topic><topic>Dielectric resonator antenna</topic><topic>Ferroelectric materials</topic><topic>Ferroelectricity</topic><topic>High temperature</topic><topic>Material chemistry</topic><topic>Permittivity</topic><topic>Perovskite materials</topic><topic>Perovskites</topic><topic>Radio antennas</topic><topic>Resonant frequencies</topic><topic>Resonators</topic><topic>Room temperature</topic><topic>Sintering (powder metallurgy)</topic><topic>Solid solutions</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Haydoura, M.</creatorcontrib><creatorcontrib>Benzerga, R.</creatorcontrib><creatorcontrib>Le Paven, C.</creatorcontrib><creatorcontrib>Le Gendre, L.</creatorcontrib><creatorcontrib>Laur, V.</creatorcontrib><creatorcontrib>Chevalier, A.</creatorcontrib><creatorcontrib>Sharaiha, A.</creatorcontrib><creatorcontrib>Tessier, F.</creatorcontrib><creatorcontrib>Cheviré, F.</creatorcontrib><collection>CrossRef</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><jtitle>Journal of alloys and compounds</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Haydoura, M.</au><au>Benzerga, R.</au><au>Le Paven, C.</au><au>Le Gendre, L.</au><au>Laur, V.</au><au>Chevalier, A.</au><au>Sharaiha, A.</au><au>Tessier, F.</au><au>Cheviré, F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications</atitle><jtitle>Journal of alloys and compounds</jtitle><date>2021-08-15</date><risdate>2021</risdate><volume>872</volume><spage>159728</spage><pages>159728-</pages><artnum>159728</artnum><issn>0925-8388</issn><eissn>1873-4669</eissn><abstract>•Synthesis of (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics with composition x between 0 and 3.•Dielectric characterization (permittivity, dielectric loss) from 10 kHz to 20 GHz.•Moderate permittivity (<100) and low dielectric loss (<8 × 10−3) at 2 GHz for x < 1.•Simulation, realization and measurement of a compact dielectric resonator antenna.•Bandwidth of 4.9% and a gain of 6.4 dB are obtained at the frequency of 5.80 GHz.
[Display omitted]
In this paper, ferroelectric ceramics with (Sr2Ta2O7)100−x(La2Ti2O7)x (STLTO) compositions have been investigated and their dielectric properties have been characterized in wide frequency band (from few kHz to few GHz); their integration in Dielectric Resonator Antennas (DRA) was conducted. The dense STLTO ceramics have been obtained by high temperature sintering of powders synthetized by solid state chemistry route. STLTO crystalline cell parameters and volume vary linearly as a function of the chemical composition (x) thus demonstrating an ideal solid solution domain for 0 ≤ x ≤ 3. Dielectric characterizations highlight that the permittivity and the dielectric loss vary according to the composition (x) and that the lowest losses are obtained for x<1.65 compositions. The latter corresponds to the transition between the ferroelectric and paraelectric compositions of the STLTO material at room temperature. A low profile DRA structure was realized using a cylindrical paraelectric STLTO resonator (with x = 0) with a permittivity of 83 and losses tanδ = 5 × 10−3@3.3 GHz. The DRA prototype was simulated, produced and tested. It exhibits a hybrid HEM11δ mode, with a resonant frequency at 5.80 GHz, a 4.9% bandwidth and a gain of 6.4 dB. These features confirm the potential of the paraelectric STLTO compositions in compact antennas radiating at frequencies below 6 GHz.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jallcom.2021.159728</doi><orcidid>https://orcid.org/0000-0002-5755-0041</orcidid><orcidid>https://orcid.org/0000-0002-2017-5233</orcidid><orcidid>https://orcid.org/0000-0001-8078-9301</orcidid><orcidid>https://orcid.org/0000-0002-5605-6113</orcidid><orcidid>https://orcid.org/0000-0002-1253-7011</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Ceramic powders Ceramics Chemical composition Chemical Sciences Dielectric loss Dielectric properties Dielectric resonator antenna Ferroelectric materials Ferroelectricity High temperature Material chemistry Permittivity Perovskite materials Perovskites Radio antennas Resonant frequencies Resonators Room temperature Sintering (powder metallurgy) Solid solutions |
title | Perovskite (Sr2Ta2O7)100−x(La2Ti2O7)x ceramics: From dielectric characterization to dielectric resonator antenna applications |
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