Electrospinning-assisted porous skeleton electrolytes for semi-solid Li-O 2 batteries

Solid-state lithium-oxygen batteries offer great promise in meeting the practical demand for high-energy-density and safe energy storage. We have developed fibrous gel polymer electrolytes (GPEs) using a polyacrylonitrile (PAN) matrix electrospinning. The 3D structure of GPEs enhances electrolyte ab...

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Published in:Chemical communications (Cambridge, England) England), 2024-05, Vol.60 (38), p.5070-5073
Main Authors: Wu, Jing, Li, Minghui, Gao, Shasha, Dou, Yaying, Pan, Kecheng, Zhang, Zhang, Zhou, Zhen
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Language:English
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cited_by cdi_FETCH-LOGICAL-c991-4f15a430e4b5e1ae535e66ce1fdfdc0049cffaff4f14759382e8147d2a538ca23
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container_issue 38
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creator Wu, Jing
Li, Minghui
Gao, Shasha
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Zhou, Zhen
description Solid-state lithium-oxygen batteries offer great promise in meeting the practical demand for high-energy-density and safe energy storage. We have developed fibrous gel polymer electrolytes (GPEs) using a polyacrylonitrile (PAN) matrix electrospinning. The 3D structure of GPEs enhances electrolyte absorption, while the interconnected design promotes strong interactions between Li and polar groups within the PAN matrix, thereby improving ion transport efficiency. In practical tests, both lithium symmetric cells and Li-O batteries demonstrated the ability to operate at high current densities over long cycles.
doi_str_mv 10.1039/D4CC00805G
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title Electrospinning-assisted porous skeleton electrolytes for semi-solid Li-O 2 batteries
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